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Graphite oxide, graphene oxide and/or graphene-containing composites for use in a filter assemblies and methods of making the same are described. Fluid treatment systems using a filter assembly having graphite oxide, graphene oxide and/or graphene-containing composites are also described. The filter assemblies and systems described herein can be used to purify contaminated fluids including water, aqueous solutions, a gas or mixture of gases, or any combination thereof. The graphite oxide, graphene oxide and/or graphene-containing composites can also have one or more of a zeolite, a boron nitride, a rare earth element, and an ionic salt incorporated therein for specific uses and desired properties.