Article including environmental barrier coating system, and method for making

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Articles for use in a high temperature environment, and methods for protecting articles in such environments, are provided. The article comprises a substrate comprising silicon; a bondcoat comprising silicon, disposed over the substrate; an intermediate barrier disposed over the bondcoat, the barrier comprising at least one layer, wherein the at least one layer comprises a rare-earth silicate and is substantially free of mullite; and a topcoat disposed over the intermediate barrier, the topcoat comprising a rare-earth monosilicate. The method comprises providing a substrate, the substrate comprising silicon; disposing a bondcoat comprising silicon over the substrate; disposing an intermediate barrier over the bondcoat, the barrier comprising at least one layer, wherein the at least one layer comprises a rare-earth silicate and is substantially free of mullite; and disposing a topcoat over the intermediate barrier, the topcoat comprising a rare-earth monosilicate.