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The present invention discloses a rare-earth sulfide colorant and a preparation method thereof. The chemical formula of the rare-earth sulfide colorant of the present invention is RE2-2xS3-3x.2y [REPO4], wherein RE is selected from one or more of La, Ce, Pr, Nd and Sm, and the ratio of y to x is 0.001 to 0.65. The present invention also discloses use of a phosphorus-containing compound for increasing the vividness of a rare-earth sulfide colorant.